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An.D. ZOLOTARENKO, Ol.D. ZOLOTARENKO, Z.A. MATYSINA, N.A. SHVACHKO, N.Y. AKHANOVA, M. UALKHANOVA, D.V. SHCHUR, M.T. GABDULLIN, Yu.I. ZHIRKO, E.P. RUDAKOVA, T.V. MYRONENKO, M.V. CHYMBAI, I.V. ZAGORULKO, and A.D. ZOLOTARENKO

Paraelectric–Ferroelectric Phase Transformations in Nanodispersed Powders of KDP Crystals
295–322 (2024)

PACS numbers: 62.20.D-, 64.60.Cn, 77.22.Ch, 77.22.Ej, 77.80.Bh, 77.84.Fa, 81.30.Hd

In the given article, a thermodynamic theory for nanodispersed powders of ferroelectrics of various structures, including KDP crystals as potential hydrogen sorbents, is presented. The article presents the statistical theory of KDP crystals developed on the basis of molecular-kinetic concepts, which allows determining, explaining and substantiating their physical properties. The temperature dependence of the order parameter, which is proportional to the degree of spontaneous polarization and deformation, is determined, and the conditions, under which a phase transition in KDP crystals turns out to be a second-order phase transformation close to a first-order one, are elucidated. The Curie temperature of the phase transition is estimated, and the dependences of the order parameter on the intensity of an external electric field or external oriented mechanical stress are established. The configurational heat capacity, its temperature dependence and jumps at the phase-transition point are estimated. The temperature dependences of the direct and inverse permittivities (or susceptibility) are determined. The validity of the Curie–Weiss law for KDP crystals is verified

KEY WORDS: nanodispersed powders, KDP crystals, ordering, Curie temperature, phase transition, molecular-kinetic concepts, ferroelectrics, ferroelastics, paraphase, ferrophase

DOI:  https://doi.org/10.15407/nnn.22.02.295

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